作者:Zhu, SY (Zhu, Songyan)[ 1,2 ] ; Li, XY (Li, Xiaoying)[ 1 ] ; Yu, C (Yu, Chao)[ 3 ] ; Wang, HM (Wang, Hongmei)[ 1,2 ] ; Wang, YP (Wang, Yapeng)[ 1,2 ] ; Miao, J (Miao, Jing)[ 1,2 ]

ATMOSPHERE

卷: 9  期: 1

文獻號: 5

DOI: 10.3390/atmos9010005

出版年: JAN 2018

摘要

The widespread distribution and strong seasonal pattern of highly concentrated summertime formaldehyde (HCHO) were observed using data from the Ozone Monitoring Instrument (OMI) onboard Aura satellite from 2005 to 2015 in Beijing-Tianjin-Hebei, China. The large-scale HCHO concentrations and its close connection with the surface O-3 pollution made the study of summertime HCHO patterns and its major contributors necessary. Accordingly, time series decomposition, Moran's I and Pearson correlation coefficient (PCC) were adopted to investigate the spatiotemporal variations of HCHO. We found that the HCHO columns regionally increased from 2005 to 2010 and decreased in the north (e.g., Chengde) from 2010 to 2015. Additionally, HCHO Vertical Column Densities (VCDs) exhibited higher values in urban areas. Despite the strong possibilities of major biogenic contributions, anthropogenic sources represented larger spatial PCCs and larger total emission rates. Industrial sources exhibited a large increasing emission amount, and the most similar distribution to HCHO was found in residential sources. By comparison, power-based emissions accounted for a relatively small fraction, and transportation emissions declined rapidly. In conclusion, anthropogenic VOCs might contribute to the summertime HCHO concentrations as well as isoprene, and controls on VOCs and HCHO would be greatly assisted by the satellite-based observations.

通訊作者地址: Li, XY (通訊作者)

Chinese Acad Sci, Inst Remote Sensing & Digital Earth, State Key Lab Remote Sensing Sci, Beijing 100101, Peoples R China.

通訊作者地址: Yu, C (通訊作者)

Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China.

地址:

[ 1 ] Chinese Acad Sci, Inst Remote Sensing & Digital Earth, State Key Lab Remote Sensing Sci, Beijing 100101, Peoples R China

[ 2 ] Univ Chinese Acad Sci, Sch Elect Elect & Commun Engn, Beijing 100049, Peoples R China

[ 3 ] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China